Heteroannulation enabled by a bimetallic Rh(iii)/Ag(i) relay catalysis: application in the total synthesis of aristolactam BII.

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ID: 90163
2017
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Ranked #13 of 184 articles by views in Chemical communications (Cambridge, England)

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Abstract
A redox-neutral bimetallic Rh(iii)/Ag(i) relay catalysis allowed the efficient construction of 3-alkylidene isoindolinones and 3-alkylidene isobenzofuranones. The Rh(iii) catalyst was responsible for the C-H monofluoroalkenylation reaction, whereas the Ag(i) salt was an activator for the follow-up cyclization. The methodology developed was applied as a key step in the rapid total synthesis of the natural product aristolactam BII.
Reference Key
ji2017heteroannulationchemical Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Ji, Wei-Wei;Lin, E;Li, Qingjiang;Wang, Honggen;
Journal Chemical communications (Cambridge, England)
Year 2017
DOI
10.1039/c7cc02105d
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Keywords
nephrotoxicity metabolomics lc-ms asarum aristolactam

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