Carbon dioxide electroreduction on single-atom nickel decorated carbon membranes with industry compatible current densities.

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ID: 89634
2020
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Abstract
Carbon dioxide electroreduction provides a useful source of carbon monoxide, but comparatively few catalysts could be sustained at current densities of industry level. Herein, we construct a high-yield, flexible and self-supported single-atom nickel-decorated porous carbon membrane catalyst. This membrane possesses interconnected nanofibers and hierarchical pores, affording abundant effective nickel single atoms that participate in carbon dioxide reduction. Moreover, the excellent mechanical strength and well-distributed nickel atoms of this membrane combines gas-diffusion and catalyst layers into one architecture. This integrated membrane could be directly used as a gas diffusion electrode to establish an extremely stable three-phase interface for high-performance carbon dioxide electroreduction, producing carbon monoxide with a 308.4 mA cm partial current density and 88% Faradaic efficiency for up to 120 h. We hope this work will provide guidance for the design and application of carbon dioxide electro-catalysts at the potential industrial scale.
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yang2020carbonnature Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Yang, Hengpan;Lin, Qing;Zhang, Chao;Yu, Xinyao;Cheng, Zhong;Li, Guodong;Hu, Qi;Ren, Xiangzhong;Zhang, Qianling;Liu, Jianhong;He, Chuanxin;
Journal Nature communications
Year 2020
DOI
10.1038/s41467-020-14402-0
URL
Keywords
tissue engineering chitin biocompatibility polysaccharide scaffold aspergillus sp. fungus glucan nano/microfibers

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