MOF Crystal Engineering Design for Cu-[O]-Ce Species in Cu-CeO2 Photoactivated Catalyst.

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ID: 83292
2020
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Abstract
Fully utilizing solar energy for catalysis requires integration of conversion mechanisms and therefore delicate design of catalyst structures and active species. Here, a MOF crystal engineering method was developed to controllably synthesize the copper-ceria catalyst with well-dispersed photoactive Cu-[O]-Ce species. Using preferential CO oxidation as a model reaction, the catalyst showed remarkably efficient and stable photoactivated catalysis, which found practical application in feed gas treatment for fuel cell gas supply. The coexistence of photochemistry and thermochemistry effects contributes to the high efficiency. Our results demonstrate a catalyst design approach with atomic or molecular precision and the combinatorial photoactivation strategy for solar energy conversion.
Reference Key
wang2020mofangewandte Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Wang, Feifan;Tian, Jie;Li, Mengzhu;Li, Weizhen;Chen, Lifang;Liu, Xiaozhi;Li, Jian;Muhetaer, Aidaer;Li, Qi;Wang, Yuan;Gu, Lin;Ma, Ding;Xu, Dongsheng;
Journal angewandte chemie (international ed in english)
Year 2020
DOI
10.1002/anie.201916049
URL
Keywords
nanoparticles photocatalysis heterogeneous catalysis metal-organic frameworks energy conversion

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