Coherent multidimensional spectroscopy of dilute gas-phase nanosystems.

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ID: 76983
2018
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Abstract
Two-dimensional electronic spectroscopy (2DES) is one of the most powerful spectroscopic techniques with unique sensitivity to couplings, coherence properties and real-time dynamics of a quantum system. While successfully applied to a variety of condensed phase samples, high precision experiments on isolated systems in the gas phase have been so far precluded by insufficient sensitivity. However, such experiments are essential for a precise understanding of fundamental mechanisms and to avoid misinterpretations. Here, we solve this issue by extending 2DES to isolated nanosystems in the gas phase prepared by helium nanodroplet isolation in a molecular beam-type experiment. This approach uniquely provides high flexibility in synthesizing tailored, quantum state-selected model systems of single and many-body character. In a model study of weakly-bound Rb and Rb molecules we demonstrate the method's unique capacity to elucidate interactions and dynamics in tailored quantum systems, thereby also bridging the gap to experiments in ultracold quantum science.
Reference Key
bruder2018coherentnature Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Bruder, Lukas;Bangert, Ulrich;Binz, Marcel;Uhl, Daniel;Vexiau, Romain;Bouloufa-Maafa, Nadia;Dulieu, Olivier;Stienkemeier, Frank;
Journal Nature communications
Year 2018
DOI
10.1038/s41467-018-07292-w
URL
Keywords
electrospinning Supercapacitor pedot: pss solid electrolyte

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