Nitrogenated holey two-dimensional structures.

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ID: 72804
2015
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Abstract
Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C2N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 10(7), with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C2N-h2D crystal has potential for use in practical applications.
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mahmood2015nitrogenatednature Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Mahmood, Javeed;Lee, Eun Kwang;Jung, Minbok;Shin, Dongbin;Jeon, In-Yup;Jung, Sun-Min;Choi, Hyun-Jung;Seo, Jeong-Min;Bae, Seo-Yoon;Sohn, So-Dam;Park, Noejung;Oh, Joon Hak;Shin, Hyung-Joon;Baek, Jong-Beom;
Journal Nature communications
Year 2015
DOI
10.1038/ncomms7486
URL
Keywords
interdigitation porous organic crystals single-crystals solid-state reactions superstructures

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