Conversion of Carbon Dioxide by Methane Reforming under Visible-Light Irradiation: Surface-Plasmon-Mediated Nonpolar Molecule Activation.

Clicks: 263
ID: 37697
2015
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Ranked #87 of 192 articles by views in angewandte chemie (international ed in english)

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Abstract
A novel CO2 photoreduction method, CO2 conversion through methane reforming into syngas (DRM) was adopted as an efficient approach to not only reduce the environmental concentration of the greenhouse gas CO2 but also realize the net energy storage from solar energy to chemical energy. For the first time it is reported that gold, which was generally regarded to be inactive in improving the performance of a catalyst in DRM under thermal conditions, enhanced the catalytic performance of Rh/SBA-15 in DRM under visible-light irradiation (1.7 times, CO2 conversion increased from 2100 to 3600 μmol g(-1) s(-1)). UV/Vis spectra and electromagnetic field simulation results revealed that the highly energetic electrons excited by local surface plasmon resonances of Au facilitated the polarization and activation of CO2 and CH4 with thermal assistance. This work provides a new route for CO2 photoreduction and offers a distinctive method to photocatalytically activate nonpolar molecules.
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liu2015conversionangewandte Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Liu, Huimin;Meng, Xianguang;Dao, Thang Duy;Zhang, Huabin;Li, Peng;Chang, Kun;Wang, Tao;Li, Mu;Nagao, Tadaaki;Ye, Jinhua;
Journal angewandte chemie (international ed in english)
Year 2015
DOI
10.1002/anie.201504933
URL
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