Topological impact of polar-gradient field constructed with laponite and surfactant for CO2 capture by spiropyran molecule

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ID: 338251
2026
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Abstract
Abstract Carbon dioxide (CO2) capture by the 1,3,3-trimethylindolinobenzopyrylospiran (TIBS) was enhanced by incorporating it into polar-gradient fields formed from laponite and hexadecyltrimethylammonium bromide (CTAB) surfactant. An increase in the CTAB concentration led sphere-to-fiber morphological transformation of the fields, stabilizing hydrophobic TIBS by suppressing isomerization to merocyanine forms. The TIBS in the fibrous fields enabled the capture of about 2 CO2 molecules per TIBS molecule. The topological engineering of the polar-gradient field is as an effective strategy for improving molecular CO2 capture by using organic dye molecules.
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Authors Masatake Mizukami, Shion Eguchi, Shuhei Shimoda, Naoki Hiratsuka, Yoshiumi Kohno, Yasumasa Tomita, Shigeo Satokawa, Keigo Tashiro
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Journal phytochemistry letters
Year 2026
DOI
10.1093/chemle/upag200
URL
https://doi.org/10.1093/chemle/upag200
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