Mechanochemical Synthesis of Fluorine-Doped NaTaCl6 Electrolytes

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ID: 319626
2026
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Abstract
Abstract Sodium-ion-conducting chlorides, particularly NaTaCl6, have attracted attention for their high ionic conductivity and oxidation stability. Here, NaTaCl6−xFx (x = 0–6) was synthesized by mechanochemical treatment to improve electrochemical stability. F doping decreased ionic conductivity, whereas NaTaCl5.75F0.25 exhibited an electrochemical potential window of 1.5–4.1 V vs. Na+/Na and stable cycling for 50 cycles at 60 °C in an all-solid-state cell. These results suggest that F doping effectively tunes the electrochemical stability of NaTaCl6-based solid electrolytes.
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Authors Takuto Magome, Kota Motohashi, Takehiro Nakao, Hirokazu Munakata, Atsushi Sakuda, A Hayashi
Journal phytochemistry letters
Year 2026
DOI
10.1093/chemle/upag143
URL
https://doi.org/10.1093/chemle/upag143
Keywords Keywords not found

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