Proximal Functionalization of Rhenium(I) Bipyridine Tricarbonyl Complexes for Photocatalytic CO2 Reduction and Carboxylation
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ID: 318118
2026
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Abstract
Abstract Two 6,6’-functionalized rhenium(I) bipyridine tricarbonyl complexes bearing hydroxy or imidazolium groups were designed and synthesized to place functional groups closer to the metal center than in the 5,5’-functionalized analogues. Single-crystal X-ray diffraction analysis confirmed the structures of these new complexes, and spectroscopic and electrochemical studies revealed the similar properties to their 5,5’-functionalized analogues. The 6,6’-functionalized complexes exhibited higher photocatalytic activity for carbon dioxide (CO2) reduction, whereas the carboxylation with CO2 was unaffected, highlighting the reaction-dependent impact of ligand functionalization.
| Reference Key |
openalex_W7165552316
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|---|---|
| Authors | Phurinat Lorwongkamol, Yutaka Saga, Shigeyuki Masaoka |
| Journal | phytochemistry letters |
| Year | 2026 |
| DOI |
10.1093/chemle/upag132
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| URL | |
| Keywords | Keywords not found |
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