Unusual Skeletal Editing of Oxadiazinones with Aryne Intermediates
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ID: 317283
2026
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Abstract
Abstract An unusual skeletal editing method involving a 6-to-8 ring expansion of oxadiazinones with aryne intermediates is disclosed. The construction of a new skeleton from oxadiazinones was confirmed by 1H and 13C NMR spectroscopy and X-ray crystallographic analysis. We found that the use of tetrabutylammonium difluorotriphenylsilicate as the activator provides access to a ring-expansion pathway distinct from the conventional Diels–Alder/denitrogenation sequence.
| Reference Key |
openalex_W7164806766
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|---|---|
| Authors | Kosuke Nagase, Yusei Yamamoto, Suguru Yoshida |
| Journal | phytochemistry letters |
| Year | 2026 |
| DOI |
10.1093/chemle/upag124
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| URL | |
| Keywords | Keywords not found |
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