Atmosphere-Dependent Hydrogen Release from Layered Hydrogen Silicane under Visible-Light Irradiation
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ID: 313345
2026
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Abstract
Abstract Layered hydrogen silicane (L-HSi) was investigated as a visible-light-responsive hydrogen carrier. Hydrogen evolution was observed under visible-light irradiation, reaching release ratios of 8% in argon and 15% in air after 7 days. Spectroscopic analyses (UV–vis, XPS, ESR) and XRD measurements revealed atmosphere-dependent structural changes. In argon, hydrogen release generates Si dangling bonds, whereas in air the dangling bonds are terminated by oxygen-containing species. These findings clarify the hydrogen release mechanism of L-HSi.
| Reference Key |
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| Authors | Mio Nakai, Kazuzshi Kiyohara, Hiroyuki Asakura, Masahiro Miyauchi, Hideyuki Nakano |
| Journal | phytochemistry letters |
| Year | 2026 |
| DOI |
10.1093/chemle/upag085
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| URL | |
| Keywords | Keywords not found |
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