some nitrogen-rich heterocycles derivatives as potential explosives and propellants: a theoretical study

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ID: 216188
2016
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Abstract
Four types of nitrogen-rich heterocycles substituted with -NO2, -NHNO2 and -C(NO2)3 explosophoric groups were explored as potential explosives and propellants materials. The calculated crystal density (ρ0)and the condensed phase heat of formation (ΔH·0f)for each of the twelve structures investigated shows that all these derivatives possess high (1.834-1.980 g cm-3)(ΔH·0f) and (605-2130 kJ kg-1) values. Interesting properties such as detonation velocity (D), pressure (P) and specific impulse (Isp) were calculated using the Kamlet-Jacobs method and ISPBKW thermochemical code. Detonation velocity and pressure in excess of 8.44 km s-1 and 32.87 GPa was obtained in all cases. Furthermore, trinitromethyl substituted derivatives shows performance exceeding that of HMX with an estimated D = 9.32-9.72 km s-1 and P = 40.61-43.82 GPa. Some -NO2 and -NHNO2 substituted derivatives were shown to be impact insensitive while retaining good detonation performance and thus are regarded as potential replacement for current RDX -based explosives. Finally, the calculated specific impulse (Isp between 248 and 270 s) of all investigated derivatives indicate that these energetic materials can be considered as possible ingredient in future rocket propellant compositions.
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Authors ;Frem Dany
Journal meditsinskaia radiologiia
Year 2016
DOI
10.2298/JSC150918002F
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