atomic charges and chemical bonding in y-ga compounds

Clicks: 115
ID: 210744
2018
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Abstract
A negative deviation from Vegard rule for the average atomic volume versus yttrium content was found from experimental crystallographic information about the binary compounds of yttrium with gallium. Analysis of the electron density (DFT calculations) employing the quantum theory of atoms in molecules revealed an increase in the atomic volumes of both Y and Ga with the increase in yttrium content. The non-linear increase is caused by the strengthening of covalent Y-Ga interactions with stronger participation of genuine penultimate shell electrons (4d electrons of yttrium) in the valence region. Summing the calculated individual atomic volumes for a unit cell allows understanding of the experimental trend. With increasing yttrium content, the polarity of the Y-Ga bonding and, thus its ionicity, rises. The covalency of the atomic interactions in Y-Ga compounds is consistent with their delocalization from two-center to multi-center ones.
Reference Key
grin2018crystalsatomic Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors ;Yuri Grin;Anatolij Fedorchuk;Rodolfo J. Faria;Frank R. Wagner
Journal turk kardiyoloji dernegi arsivi
Year 2018
DOI
10.3390/cryst8020099
URL
Keywords Keywords not found

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