systematic reduction of the detailed kinetic mechanism for the combustion of n-butane
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ID: 197915
2016
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Abstract
A systematic approach for mechanism reduction was demonstrated to generate a skeletal and reduced mechanism for the oxidation of n-butane. First, a skeletal mechanism, including 89 species and 440 elementary reactions, was derived from a 230-species detailed mechanism using path flux analysis (PFA). Then, the unimportant reactions were eliminated using the importance index defined in computational singular perturbation (CSP), resulting in a skeletal mechanism consisting of 89 species and 298 elementary reactions. Finally, 20 global quasi-steady-state species were identified using a CSP-based time-scale analysis, leading to a 69-species reduced mechanism. Validation of the 89-species skeletal and 69-species reduced mechanisms showed good agreement with the detailed mechanism for both the ignition delay time and the distribution of species concentration over a wide range of simulation conditions.
| Reference Key |
liu2016journalsystematic
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|---|---|
| Authors | ;Chunhui Liu;Zhengxing Zuo;Huihua Feng |
| Journal | british journal of psychology (london, england : 1953) |
| Year | 2016 |
| DOI |
10.1155/2016/8153582
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| URL | |
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