growing of CoO nanoparticles on g-CN composites with highly improved photocatalytic activity for hydrogen evolution.
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2019
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Abstract
CoO/g-CN hybrid catalyst is facilely prepared for application to photocatalytic H evolution from water splitting by the vacuum rotation-evaporation and thermal method. The physical and chemical properties of CoO/g-CN are determined by a series of characterization methods. The g-CN with 0.6 wt% Co loading exhibits superior photocatalytic hydrogen evolution activity with an H evolution amount of 23.25 mmol g after 5 h. The obtained 0.6 wt% CoO/g-CN can split water to generate 0.39 mmol g H without sacrificial agent and noble metal, while the pure g-CN is inactive under the same reaction conditions. The remarkable enhancement of photocatalytic H evolution activity of CoO/g-CN composites is mainly ascribed to the effective separation of electron-hole pairs and charge transfer. The work creates new opportunities for the design of low-cost g-CN-based photocatalysts with high photocatalytic H evolution activity from overall water splitting.
| Reference Key |
liu2019royal
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| Authors | Liu, Xuecheng;Zhang, Qian;Liang, Liwei;Chen, Lintao;Wang, Yuyou;Tan, Xiaoqing;Wen, Li;Huang, Hongyu; |
| Journal | Royal Society open science |
| Year | 2019 |
| DOI |
10.1098/rsos.190433
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| URL | |
| Keywords | Keywords not found |
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