complete bromide surface segregation in mixed nacl/nabr aerosols grown from droplets
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2015
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Abstract
Sea-salt aerosols are a source of atmospheric bromine responsible for ozone depletion. The availability of bromine from sea-salt aerosols to heterogeneous phase chemical reactions is determined by its local concentration at the aerosol surface. We report here complete surface segregation of bromine in mixed NaCl/NaBr aerosols grown by drying droplets, thus mimicking the atmospheric process by which solid sea-salt aerosols are generated. For d=70 nm solid aerosols, complete surface segregation is observed for solution Br/Cl ratios below 2%. These findings set a size-dependent upper limit on the bromine surface enrichment that can be reached in solid salt aerosols grown from sea-water droplets in the atmosphere.
| Reference Key |
antonsson2015physicalcomplete
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|---|---|
| Authors | ;Egill Antonsson;Minna Patanen;Christophe Nicolas;John J. Neville;Safia Benkoula;Alok Goel;Catalin Miron |
| Journal | american journal of transplantation |
| Year | 2015 |
| DOI |
10.1103/PhysRevX.5.011025
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| URL | |
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