Divergent Chemistry Paths for 3D and 1D Metallo-Covalent Organic Frameworks.

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ID: 102986
2020
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Abstract
The marriage of dynamic covalent chemistry (DCC) and coordination chemistry is a powerful tool for assembling complex architectures from simple building units. Recently, the synthesis of woven covalent organic frameworks (COFs) with topologically fascinating structures has been achieved using this approach. However, the scope is highly limited and there is a need to discover new pathways that can assemble covalently linked organic threads into crystalline frameworks. Here, we have identified branching pathways leading to the assembly of three-dimensional (3D) woven COFs or one-dimensional (1D) metallo-COFs (mCOFs), where the mechanism is underpinned by the absence or presence of ligand exchange.
Reference Key
xu2020divergentangewandte Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Xu, Hai-Sen;Luo, Yi;See, Pei Zhen;Li, Xing;Chen, Zhongxin;Zhou, Yi;Zhao, Xiaoxu;Leng, Kai;Park, In-Hyeok;Li, Runlai;Liu, Cuibo;Chen, Fangzheng;Xi, Shibo;Sun, Junliang;Loh, Kian Ping;
Journal angewandte chemie (international ed in english)
Year 2020
DOI
10.1002/anie.202002724
URL
Keywords
structure elucidation covalent organic frameworks 3d and 1d metal templates self assembly

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