Nanowire Array-Coated Flexible Substrate to Accommodate Lithium Plating for Stable Lithium-Metal Anodes and Flexible Lithium-Organic Batteries.

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ID: 39398
2019
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Abstract
Although lithium metal is an ideal anode with high theoretical capacity, Li dendrite formation and volume change have limited its application. We report a vertical polyaniline nanowire-coated carbon nanotube (CNT/PANI) composite flexible electrode on which Li could be homogeneously deposited to obtain a CNT/PANI@Li anode. In the composite, CNT/PANI acted as a host matrix with well-distributed Li ion flux attributed to high electroactive surface area, thereby effectively suppressing the Li dendrite. Compared with the pure CNT electrode, the CNT/PANI electrode presented low overpotential and stable long-term cycling with much less fluctuant stripping/plating profiles. The potential application of CNT/PANI@Li in all-flexible full cells was demonstrated by combining flexible organic poly(2,5-dihydroxyl-1,4-benzoquinonyl sulfide)/carbon nanotube (PDHBQS/CNT) composite films, in which the cathode achieves an eminent performance of 120 mA h g at 50 mA g. Furthermore, pouch batteries with good flexibility were tested successfully, which demonstrated a promising future for all-flexible and high-performance Li-metal batteries.
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zhang2019nanowireacs Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Zhang, Miao;Lu, Ruichao;Yuan, Hongxin;Amin, Kamran;Mao, Lijuan;Yan, Wei;Wei, Zhixiang;
Journal ACS applied materials & interfaces
Year 2019
DOI
10.1021/acsami.9b05056
URL
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