An insight into clustering of halogenated anesthetics molecules in metal-organic frameworks: Evidence of adsorbate self-association in micropores.

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ID: 3909
2019
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Abstract
In order to better understand the adsorption of volatile halogenated anesthetics on metal organic frameworks (MOFs), sevoflurane vapor adsorption experiments were performed on commercial MOF-177 at different temperatures. Due to the surface homogeneity of such an adsorbent, arising from its almost unimodal pore size distribution and the absence of specific, coordinatively unsaturated adsorption active sites, sevoflurane adsorption isotherms exhibited a peculiar deviation from the Langmuirian behavior. Consequently, they show a "kink" at a specific pressure that increases with increasing equilibrium temperature. Successful modeling of such data by means of the Talu-Meunier equation confirmed clustering of adsorbate molecules inside adsorbent micropores, similarly to water vapor adsorption on activated carbon, which may play an important role when designing a system using MOFs as the potential adsorbents for capturing anesthetics.
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gargiulo2019anjournal Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Gargiulo, Nicola;Peluso, Antonio;Aprea, Paolo;Eić, Mladen;Caputo, Domenico;
Journal Journal of colloid and interface science
Year 2019
DOI
S0021-9797(19)30812-4
URL
Keywords Keywords not found

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