Predicting molecular scale skin-effect in electrochemical impedance due to anomalous subdiffusion mediated adsorption phenomenon

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ID: 33256
2016
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Abstract
Anomalous subdiffusion governs the processes which are not energetically driven, on a molecular scale. This paper proposes a model to predict the response of electrochemical impedance due to such diffusion process. Previous works considered the use of fractional calculus to predict the impedance behaviour in response to the anomalous diffusion. Here, we have developed an expression which predicts the skin-effect, marked by an increase in the impedance with increasing frequency, in this regime. Negative inductances have also been predicted as a consequence of the inertial response of adsorbed species upon application of frequency-mediated perturbations. It might help the researchers in the fields of impedimetric sensors to choose the working frequency and those working in the field of batteries to choose the parameters, likewise. This work would shed some light into the molecular mechanisms governing the impedance when exposed to frequency-based perturbations like electromagnetic waves (microwaves to ionizing radiations) and in charge storage devices like batteries etc.
Reference Key
kushagra2016predictingaip Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Kushagra, A.
Journal aip advances
Year 2016
DOI
10.1063/1.4942205
URL
http://dx.doi.org/10.1063/1.4942205
Keywords Keywords not found

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