Charge Density Wave Melting in One-Dimensional Wires with Femtosecond Subgap Excitation.
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ID: 29252
2019
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Abstract
Charge density waves (CDWs) are symmetry-broken ground states that commonly occur in low-dimensional metals due to strong electron-electron and/or electron-phonon coupling. The nonequilibrium carrier distribution established via photodoping with femtosecond laser pulses readily quenches these ground states and induces an ultrafast insulator-to-metal phase transition. To date, CDW melting has been mainly investigated in the single-photon regime with pump photon energies bigger than the gap size. The recent development of strong-field midinfrared sources now enables the investigation of CDW dynamics following subgap excitation. Here we excite prototypical one-dimensional indium wires with a CDW gap of ∼300 meV with midinfrared pulses at ℏω=190 meV with MV/cm field strength and probe the transient electronic structure with time- and angle-resolved photoemission spectroscopy. We find that the CDW gap is filled on a timescale short compared to our temporal resolution of 300 fs and that the band structure changes are completed within ∼1 ps. Supported by a minimal theoretical model we attribute our findings to multiphoton absorption across the CDW gap.
| Reference Key |
chvezcervantes2019chargephysical
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|---|---|
| Authors | Chávez-Cervantes, M;Topp, G E;Aeschlimann, S;Krause, R;Sato, S A;Sentef, M A;Gierz, I; |
| Journal | physical review letters |
| Year | 2019 |
| DOI |
10.1103/PhysRevLett.123.036405
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| URL | |
| Keywords | Keywords not found |
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