A Methylthio-Functionalized-MOF Photocatalyst with High Performance for Visible-Light-Driven H2 Evolution

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ID: 272069
2018
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Abstract
Recently, the emergence of photoactive metal–organic frameworks (MOFs) has given great prospects for their applications as photocatalytic materials in visible‐light‐driven hydrogen evolution. Herein, a highly photoactive visible‐light‐driven material for H2 evolution was prepared by introducing methylthio terephthalate into a MOF lattice via solvent‐assisted ligand‐exchange method. Accordingly, a first methylthio‐functionalized porous MOF decorated with Pt co‐catalyst for efficient photocatalytic H2 evolution was achieved, which exhibited a high quantum yield (8.90 %) at 420 nm by use sacrificial triethanolamine. This hybrid material exhibited perfect H2 production rate as high as 3814.0 μmol g−1 h−1, which even is one order of magnitude higher than that of the state‐of‐the‐art Pt/MOF photocatalyst derived from aminoterephthalate.
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Authors Shu-Yan Han,Dong-Lai Pan,Hui Chen,Xian-Bao Bu,Yi-Xuan Gao,Hui Gao,Yang Tian,Gui-Sheng Li,Guo Wang,Sheng-Li Cao,Chong-Qing Wan,Guo-Cong Guo;Shu-Yan Han;Dong-Lai Pan;Hui Chen;Xian-Bao Bu;Yi-Xuan Gao;Hui Gao;Yang Tian;Gui-Sheng Li;Guo Wang;Sheng-Li Cao;Chong-Qing Wan;Guo-Cong Guo;
Journal zeitschrift für angewandte chemie
Year 2018
DOI
10.1002/ange.201806077
URL
https://sciprofiles.com/publication/view/cc15f5fe15e3ffb141e202653e387fb9
Keywords
metall-organische gerüststrukturen methylthio-funktionalisierung photokatalysatoren sichtbares licht wasserstoffentwicklung

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