MULTISITE ADSORPTION AND ORDER-DISORDER TRANSITIONS IN ONE- AND TWO-DIMENSIONAL PHASES CONDENSED ON FOREIGN SUBSTRATE

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ID: 270424
1977
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Abstract
Isotherms and free energy variations at equilibrium in the case of fixed one-to-n adsorption (i.e. the average occupation of n adsorption sites by one adsorbed molecule) are calculated for one-dimensional models and their properties are discussed. It proceeds that no first order transition can be expected between a condensed (one-to-n) disordered phase and the ordered (one-to-one) solid phase. Configurational entropy of an adsorbed two-dimensional one-to-n phase is computed numerically during a random sequential filling simulation. Since in this case, the two-dimensional phase is built in a disordered manner, the system can swing abruptly from disordered to ordered state.
Reference Key
bonissent1977journalmultisite Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors B. Mutaftschiev,A. Bonissent;B. Mutaftschiev;A. Bonissent;
Journal journal de physique iv (proceedings)
Year 1977
DOI
10.1051/jphyscol:1977413
URL
https://sciprofiles.com/publication/view/a5121bfa4cc05ec51de8dc007683be25
Keywords
foreign substrate multisite adsorption phases condensed dimensional phases adsorption and order disorder transitions

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