Catalytic Cyclopropanation by Myoglobin Reconstituted with Iron Porphycene: Acceleration of Catalysis due to Rapid Formation of the Carbene Species

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ID: 268893
2017
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Abstract
Myoglobin reconstituted with iron porphycene catalyzes the cyclopropanation of styrene with ethyl diazoacetate. Compared to native myoglobin, the reconstituted protein significantly accelerates the catalytic reaction and the kcat/Km value is 26-fold enhanced. Mechanistic studie …
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Authors Oohora K;Meichin H;Zhao L;Wolf MW;Nakayama A;Hasegawa JY;Lehnert N;Hayashi T;;
Journal Journal of the American Chemical Society
Year 2017
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