Merging Visible Light with Cross-Coupling: The Photochemical Direct C-H Difluoroalkylation of Imidazopyridines.

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ID: 26447
2019
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Abstract
A transition-metal-free protocol for the difluoroalkylation of imidazopyridines with bromodifluoroaryl ketones promoted by visible light irradiation is presented. This protocol is distinguished by simple, mild, and catalyst-free reaction conditions with a wide reaction scope, which is complementary to existing difluoroalkylation strategies by photoredox scenarios. Additionally, this protocol potentially offers a new way for streamlining the synthesis of compounds containing the difluoro moiety.
Reference Key
qu2019mergingorganic Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Qu, Chuan-Hua;Song, Gui-Ting;Xu, Jia;Yan, Wei;Zhou, Cheng-He;Li, Hong-Yu;Chen, Zhong-Zhu;Xu, Zhi-Gang;
Journal Organic letters
Year 2019
DOI
10.1021/acs.orglett.9b02487
URL
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