Scalable and Universal Route for the Deposition of Binary, Ternary, and Quaternary Metal Sulfide Materials from Molecular Precursors.

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ID: 263633
2020
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Abstract
A range of binary, ternary (CFS), and quaternary (CZTS) metal sulfide materials have been successfully deposited onto the glass substrates by air-spray deposition of metal diethyldithiocarbamate molecular precursors followed by pyrolysis (18 examples). The as-deposited materials were characterized by powder X-ray diffraction (p-XRD), Raman spectroscopy, secondary electron microscopy (SEM), and energy-dispersive X-ray (EDX) spectroscopy, which in all cases showed that the materials were polycrystalline with the expected elemental stoichiometry. In the case of the higher sulfides, EDX spectroscopy mapping demonstrated the spatial homogeneity of the elemental distributions at the microscale. By using this simple and inexpensive method, we could potentially fabricate thin films of any given main group or transition metal chalcogenide material over large areas, theoretically on substrates with complex topologies.
Reference Key
murtaza2020scalableacs Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Murtaza, Ghulam;Alderhami, Suliman;Alharbi, Yasser T;Zulfiqar, Usama;Hossin, Mousa;Alanazi, Abdulaziz M;Almanqur, Laila;Onche, Emmanuel Usman;Venkateswaran, Sai P;Lewis, David J;
Journal ACS applied energy materials
Year 2020
DOI
10.1021/acsaem.9b02359
URL
Keywords
hydrogen peroxide heterogeneous catalysis degradation sulfadiazine cu(2)znsns(4)

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