tropospheric ozone maxima observed over the arabian sea during the pre-monsoon
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2017
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Abstract
An enhancement of the tropospheric ozone column (TOC) over Arabian Sea (AS)
during the pre-monsoon season is reported in this study. The potential
sources of the AS spring ozone pool are investigated by use of multiple data
sets (e.g., SCIAMACHY Limb-Nadir-Matching TOC, OMI/MLS TOC, TES TOC, MACC
reanalysis data, MOZART-4 model and HYSPLIT model). Three-quarters of the enhanced ozone
concentrations are attributed to the 0–8 km height range. The main source
of the ozone enhancement is considered to be caused by long-range transport
of ozone pollutants from India (∼ 50 % contributions to the lowest
4 km, ∼ 20 % contributions to the 4–8 km height range), the
Middle East, Africa and Europe (∼ 30 % in total). In addition, the
vertical pollution accumulation in the lower troposphere, especially at
4–8 km, was found to be important for the AS spring ozone pool formation.
Local photochemistry, on the other hand, plays a negligible role in producing
ozone at the 4–8 km height range. In the 0–4 km height range, ozone is
quickly removed by wet deposition. The AS spring TOC maxima are influenced by
the dynamical variations caused by the sea surface temperature (SST) anomaly
during the El Niño period in 2005 and 2010 with a ∼ 5 DU decrease.
| Reference Key |
jia2017atmospherictropospheric
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|---|---|
| Authors | ;J. Jia;A. Ladstätter-Weißenmayer;X. Hou;A. Rozanov;J. P. Burrows |
| Journal | Journal of agricultural and food chemistry |
| Year | 2017 |
| DOI |
10.5194/acp-17-4915-2017
|
| URL | |
| Keywords |
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