The Special "Morse Code" between Solvent Polarity and Morphology Flexibility in in POSS-dendrimer supramolecular system.

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ID: 2263
2019
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Abstract
An amazing phenomenon of the relative magnitude of modulus of two liquid crystal (LC) gels is found inverted under/above their phase transition temperature TLC-iso, which is further proved to be caused by their diverse morphology flexibility. By testing the polarity of two LCs, we discovered that gelator POSS-G1-Boc self-assemble into more flexible structures in a relative low polar LC, while more rigid ones are formed in higher polar LC. Hence we established a fitting function to connect morphology flexibility with solvent polarity, which can even be generalized to a number of common solvents. Experimental observations and coarse-grained molecular dynamics simulations revealed that solvent polarity is just like the special "morse code", and each "morse code" corresponding to a specific morpholsogy flexibility.
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shan2019thechemistry Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Tianyu Shan, Liang Gao, Xiaoqian Tong, Qinqing Du, Zhihang An, Huiwen He, Jiaping Lin, Si Chen, Xu Wang
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Journal Chemistry (Weinheim an der Bergstrasse, Germany)
Year 2019
DOI
10.1002/chem.201901422
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