ultrafast charge transfer visualized by two-dimensional electronic spectroscopy
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ID: 222820
2013
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Abstract
Two-dimensional electronic spectroscopy (2D-ES) is used to investigate ultrafast excited-state dynamics in a lutetium bisphthalocyanine dimer. Following optical excitation, a chain of electron and hole transfer steps gives rise to characteristic cross-peak dynamics in the electronic 2D spectra. The combination of density matrix propagation and quantum chemical calculations results in a molecular view of the charge transfer dynamics and highlights the role of the counter-ion in providing an energetic perturbation which promotes charge transfer across the complex.
| Reference Key |
t.2013epjultrafast
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|---|---|
| Authors | ;Mančal T.;Milota F.;Hauer J.;Christensson N.;Bixner O.;Lukeš V.;Kauffmann H. F. |
| Journal | utilitas mathematica |
| Year | 2013 |
| DOI |
10.1051/epjconf/20134108019
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