characterization and electrocatalytic properties of titanium-based ru0.3co0.7−xcex mixed oxide electrodes for oxygen evolution in alkaline solution
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ID: 219730
2011
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Abstract
Ti-supported RuO2-Co3O4-CeO2
(Ru0.3Co0.7−xCex oxide, 0≤x≤0.7) electrodes were prepared by sol-gel process. The phase structure, surface morphology, and microstructure of the oxide layer were characterized by X-ray diffraction (XRD) and scanning electron microscopy (SEM). Electrocatalytic activity and oxygen evolution reaction (OER) kinetics on these electrodes in 1.0 mol⋅dm−3 KOH solution were studied by recording open-circuit potential, cyclic voltammetry, and polarisation curves. The results showed that the appropriate content of CeO2 could reduce the grain size and increase active surface area. The electrocatalytic activity shows a strong dependence on the CeO2 content in the film. Catalytic performance of mixed oxide electrodes with 40 mol % CeO2 was the best, with the greatest voltammetric charge, 86.23 mC⋅cm−2, and the smallest apparent activation energy for OER at 0.60 V was 22.76 kJ⋅mol−1.
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wu2011journalcharacterization
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|---|---|
| Authors | ;Hongjun Wu;Qin Ruan;Li Li;Baohui Wang |
| Journal | reproductive biology and endocrinology |
| Year | 2011 |
| DOI |
10.1155/2011/624067
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