iminoiodane- and brønsted base-mediated cross dehydrogenative coupling of cyclic ethers with 1,3-dicarbonyl compounds

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ID: 213772
2015
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Abstract
A one-pot, two-step approach to prepare 2-tetrahydrofuran and -pyran substituted 1,3-dicarbonyl compounds by PhI=NTs-mediated amination/Brønsted base-catalyzed cross dehydrogenative coupling (CDC) reaction of the cyclic ether and 1,3-dicarbonyl derivative under mild conditions is reported. The reaction is compatible with a variety of cyclic ethers and 1,3-dicarbonyl compounds, affording the corresponding coupled products in moderate to good yields of up to 80% over two steps.
Reference Key
tejo2015moleculesiminoiodane- Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors ;Ciputra Tejo;Xiao Rong Sim;Bo Ra Lee;Benjamin James Ayers;Chung-Hang Leung;Dik-Lung Ma;Philip Wai Hong Chan
Journal Journal of ethnopharmacology
Year 2015
DOI
10.3390/molecules200713336
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