in-situ liquid hydrogenation of m-chloronitrobenzene over fe-modified pt/carbon nanotubes catalysts
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ID: 212644
2018
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Abstract
In-situ liquid-phase hydrogenation of m-chloronitrobenzene (m-CNB) based on aqueous-phase reforming (APR) of ethanol and catalytic hydrogenation was carried out over Fe-modified Pt/carbon nanotubes (CNTs) catalysts. The effects of Pt loading over CNTs and Fe modification on the catalytic performance of Pt/CNTs catalysts were studied. In-tube loading of Pt particles, compared with out-tube loading, considerably improved the catalytic activity. With in-tube loading, Fe-modified Pt/CNTs catalysts further improved the m-CNB in-situ hydrogenation performance. After Fe modification, Pt–Fe/CNTs catalysts formed, inside CNTs, a Pt–Fe alloy and iron oxides, which both improved catalytic hydrogenation performance and significantly enhanced ethanol APR hydrogen producing performance, thereby increasing the m-CNB in-situ hydrogenation reactivity.
| Reference Key |
li2018catalystsin-situ
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|---|---|
| Authors | ;Feng Li;Jinrong Liang;Wenxi Zhu;Hua Song;Keliang Wang;Cuiqin Li |
| Journal | journal of essential oil research |
| Year | 2018 |
| DOI |
10.3390/catal8020062
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| URL | |
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