two chemically stable cd(ii) polymers as fluorescent sensor and photocatalyst for aromatic dyes
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ID: 189057
2018
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Abstract
Two new 2D Cd(II)-based coordination polymers (CPs), viz. [Cd2(H2L)2(2,2’-bipy)2] (1) and [Cd(L)0.5(phen)·0.5H2O] (2), have been constructed using ethylene glycol ether bridging tetracarboxylate ligand 5,5′(4,4′-phenylenebis(methyleneoxy)) diisophthalic acid (H4L). Both CPs behaved as profound fluorescent sensor for Fe3+ ion and nitro-aromatics (NACs), specifically 2,4,6-trinitrophenol (TNP). The stability at elevated temperature and photocatalytic behaviors of both 1 and 2 for photo-decomposition of aromatic dyes have also been explored. An attempt has been made to explore the plausible mechanism related with the decrease in fluorescence intensity of 1 and 2 in presence of NACs using theoretical calculations. Additionally, the probable mechanism of photo catalysis by 1 and 2 to photo-degrade aromatic dyes has been explained using density of states (DOS) calculations.
| Reference Key |
wang2018polymerstwo
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|---|---|
| Authors | ;Jun Wang;Jian Wu;Lu Lu;Ai-Qing Ma;Wan-Shan Hu;Wei-Ping Wu;Yu Wu;Yan-Chun Sun;Amita Singh;Abhinav Kumar |
| Journal | Journal of Fluorescence |
| Year | 2018 |
| DOI |
10.3390/polym10030274
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