base-free selective oxidation of glycerol over ldh hosted transition metal complexes using 3% h2o2 as oxidant

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ID: 187139
2016
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Abstract
A series of transition metal sulphonato-Schiff base complexes were intercalated into Mg–Al layered-double hydroxides (LDHs). The obtained catalysts were characterized by FTIR, XRD, N2 sorption, SEM and elemental analysis, and then were used in the selective oxidation of glycerol (GLY) using 3% H2O2 as an oxidant. It was found that their catalytic performances were closely related to the loading of active complexes, the Schiff base ligands and the metal centers of the catalysts, as well as the reaction conditions. The optimal conversion of GLY was 85.0%, while the selectivity of 1,3-dihydroxyacetone (DHA) was 56.5%. Moreover, the catalysts could be reused at least 10 times.
Reference Key
wang2016catalystsbase-free Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors ;Xiaoli Wang;Congxiao Shang;Gongde Wu;Xianfeng Liu;Hao Liu
Journal journal of essential oil research
Year 2016
DOI
10.3390/catal6070101
URL
http://www.mdpi.com/2073-4344/6/7/101
Keywords
transition metal selective oxidation ldh

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