All-Solid-State Lithium Organic Batteries Comprising Single-Ion Polymer Nanoparticle Electrolytes.

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ID: 101151
2020
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Abstract
Advances in lithium battery technologies necessitate improved energy densities, long cycle lives, fast charging, safe operation, and environment-friendly components. In this study, we investigated lithium organic batteries comprising bioinspired polyvinyl catechol (P4VC) cathode materials and single-ion conducting polymer nanoparticle electrolytes. The controlled synthesis of P4VC resulted in a two-step redox reaction with voltage plateaus at ~3.1 and ~3.5 V as well as a high initial specific capacity of 352 mAh g -1 . The use of single-ion nanoparticle electrolytes enabled the synergistic achievement of high electrochemical stabilities up to 5.5 V, lithium transference number of 0.87, high ionic conductivities ranging from 0.2 × 10 -3 to 10 -3 S cm -1 , and stable storage moduli >10 MPa in 25-90 °C. Lithium cells can deliver 165 mAh g -1 at 39.7 mA g -1 for 100 cycles and stable specific capacity >100 mAh g -1 at high current density of 794 mA g -1 for 500 cycles. As the first successful demonstration of solid-state single-ion polymer electrolytes in environmentally benign and cost-effective lithium organic batteries, this work establishes a future research avenue for advancing lithium battery technologies.
Reference Key
kim2020allsolidstatechemsuschem Use this key to autocite in the manuscript while using SciMatic Manuscript Manager or Thesis Manager
Authors Kim, Boram;Kang, Haneol;Kim, Kyoungwook;Wang, Rui-Yang;Park, Moon Jeong;
Journal ChemSusChem
Year 2020
DOI
10.1002/cssc.202000117
URL
Keywords
nanoparticles electrochemistry polymer electrolytes lithium-organic batteries single-ion polymers

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